This paper aims to discuss the dynamic adsorption processes of carbon dioxide in a porous fixed bed on the industrial scale, using a multiple-relaxation-time lattice Boltzmann (LB) model.
A multiple-relaxation-time LB model is developed to predict the dynamic adsorption processes of carbon dioxide in a porous fixed bed on the industrial scale. The breakthrough curves from the simulation results are compared with the experimental data to validate the reliability of this model, and the effects of flow velocity, porosity and linear driving force mass transfer coefficient on the adsorption behaviors of carbon dioxide are explored further.
The numerical results show that the improved fluid flux leads to the reduction in the time required for completion of adsorption processes nonlinearly, and the differential pressure significantly raises with the decreasing porosity of porous fixed bed for fixed values of Reynolds number and total adsorption capacity. The maximum adsorption ratio of carbon dioxide was found at Re = 12 in this work. In addition, the higher mass transfer resistance of adsorbent particles advances the appearance time of the breakthrough point and delays the completion time of the adsorption processes.
This work will provide a way to study the adsorption technology of carbon dioxide in the fixed-bed using the LB method.
