The viability of converting recycled concrete fines (RCF) into low-grade artificial limestone, through carbonation in aqueous systems, for use as a sustainable replacement for high-grade limestone in limestone–calcined clay cement (LC3) was explored. The experimental results suggest that the carbonated RCF (CRCF) exhibited high pozzolanic activity, generating additional calcium (aluminium) silicate hydrate (C-(A)-S-H) to serve as nucleation sites for LC3 hydration. The refined particle size of the CRCF and the presence of fine-sized calcium carbonate further facilitated initial ions dissolution, accelerating early-age hydration and improving the pore structure of the LC3. Moreover, the incorporation of CRCF significantly enhanced the compressive strength of the LC3. Specially, when CRCF were used as a complete replacement of limestone, the compressive strength improved by 19.82% at 3 days and 2.50% at 28 days, respectively, relative to the control. These findings demonstrate the potential of CRCF as a sustainable alternative to limestone, contributing to both efficient concrete waste utilisation and environmentally friendly LC3 production.
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1 December 2025
Research Article|
November 17 2025
Effect of carbonated recycled concrete fines on the performance of limestone–calcined clay cement Available to Purchase
Yingyu Wang;
Yingyu Wang
School of Civil Engineering and Architecture,
Anhui University of Science and Technology
, Huainan, China
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Peiyuan Chen;
Peiyuan Chen
Joint National–Local Engineering Research Centre for Safe and Precise Coal Mining,
Anhui University of Science and Technology
, Huainan, China
; School of Civil Engineering and Architecture, Anhui University of Science and Technology, Huainan, China
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Zijian Zong;
Zijian Zong
School of Civil Engineering and Architecture,
Anhui University of Science and Technology
, Huainan, China
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Jin Li;
Jin Li
School of Civil Engineering and Architecture,
Anhui University of Science and Technology
, Huainan, China
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Jingjing Fang;
Jingjing Fang
School of Civil Engineering and Architecture,
Anhui University of Science and Technology
, Huainan, China
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Aiguo Wang
Anhui Province Engineering Laboratory of Advanced Building Materials,
Anhui Jianzhu University
, Hefei, China
; Anhui Province Key Laboratory of Advanced Building Materials, Anhui Jianzhu University, Hefei, ChinaCorresponding author Aiguo Wang (wag3134@126.com)
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Corresponding author Aiguo Wang (wag3134@126.com)
Declaration of competing interests The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
Publisher: Emerald Publishing
Received:
June 23 2025
Accepted:
August 25 2025
Online ISSN: 1751-763X
Print ISSN: 0024-9831
Funding
Funding Group:
- Award Group:
- Funder(s): National Natural Science Foundation of China
- Award Id(s): 52227901,52008003
- Funder(s):
- Award Group:
- Funder(s): Outstanding Youth Projects of Natural Science Research in Universities of Anhui Province
- Award Id(s): 23AH030043
- Funder(s):
- Award Group:
- Funder(s): Open Research Grant of Joint National–Local Engineering Research Centre for Safe and Precise Coal Mining
- Award Id(s): EC2023010
- Funder(s):
- Award Group:
- Funder(s): Open Research Grant of Key Laboratory of Xinjiang Coal Resources Green Mining
- Award Id(s): KLXGY-KB2417
- Funder(s):
- Award Group:
- Funder(s): Anhui Provincial Science and Technology Innovation Key Projects Plan
- Award Id(s): 202423110050008
- Funder(s):
- Award Group:
- Funder(s): Tongling Municipal Science and Technology Plan Project
- Award Id(s): 20230203048
- Funder(s):
- Award Group:
- Funder(s): University Synergy Innovation Program of Anhui Province
- Award Id(s): GXXT-2023-061
- Funder(s):
- Funding Statement(s): The authors acknowledge the National Natural Science Foundation of China (52227901 and 52008003), Outstanding Youth Projects of Natural Science Research in Universities of Anhui Province (23AH030043), Open Research Grant of Joint National–Local Engineering Research Centre for Safe and Precise Coal Mining (EC2023010), Open Research Grant of Key Laboratory of Xinjiang Coal Resources Green Mining (KLXGY-KB2417), Anhui Provincial Science and Technology Innovation Key Projects Plan (202423110050008), Tongling Municipal Science and Technology Plan Project (20230203048) and the University Synergy Innovation Program of Anhui Province (No. GXXT-2023-061). Thanks also go to the Analytical and Testing Center of Anhui University of Science and Technology for help in sample analysis.
© 2025 Emerald Publishing Limited
2025
Emerald Publishing Limited
Licensed re-use rights only
Magazine of Concrete Research (2025) 77 (23-24): 1351–1362.
Article history
Received:
June 23 2025
Accepted:
August 25 2025
Citation
Wang Y, Chen P, Zong Z, Li J, Fang J, Wang A (2025), "Effect of carbonated recycled concrete fines on the performance of limestone–calcined clay cement". Magazine of Concrete Research, Vol. 77 No. 23-24 pp. 1351–1362, doi: https://doi.org/10.1680/jmacr.25.00247
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